University Rostock Researchers Studied Atoms Molecules Interactions Biochemical Reactions

Scientists provide details of interactions on the atomic scale

11:34 AM, 26th August 2013
University of Rostock Research NEws
The image demonstrates the principle of measurement which enables to address atom-specific and state-dependent emission of photons.

BERLIN, GERMANY: How exactly atoms and molecules in biochemical solutions or at solid-liquid interfaces do interact, is a question of great importance. Answers will provide insights at processes in catalysts, smart functional materials and even physiological processes in the body, which are essential for health. Until now, scientists could have a look at these interactions by methods of spectroscopy, but it was hard to distinguish the many different interactions, which take place simultaneously.

A groundbreaking work by HZB-scientists could now change the game. Dr Emad Flear Aziz, Professor, HZB and his team provides a new tool, which enables scientists to get a “fingerprint” of the interactions on the atomic scale. In collaboration with the group of theoretical physicist Oliver Kuhn, University of Rostock these fingerprints can be interpreted and linked to specific chemical interactions, thus allowing direct insight in what happens in the former ‘black box.’

“Basically we are looking at how atoms and molecules interact in biochemical materials in solution,” said Aziz. The work is based on a discovery by Aziz’ team made three years before: They then analyzed samples with x-ray spectroscopy and observed the disappearance of photons at some specific photon energy. These results have been replicated by other teams worldwide. To explain this effect, Aziz and colleagues proposed a “dark channel mechanism,” which should provide information about binding processes and interactions between atoms or molecules. This explanation stirred a big debate among scientists.

In order to understand, how the spectral findings are linked to binding and structural processes inside the sample, Oliver Kuhn and his postdoc Sergey Bokarev provided a theoretical tool, based on ab initio calculations of energy levels inside the molecules.  “We can map all electronic states in the systems we probe, and we can distinguish those which are involved in building bonds with neighbours from those which are not involved,” explained Aziz.

Metaphorically speaking, if the interacting molecules produce a sort of party chatter, the scientists are now able to listen to specific conversations. They are convinced that these new tools will bring deeper insights into the chemistry of life.

© HZB News

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